Frou Frou - Let Go headline track on the album; used in the soundtrack to Garden State.
Frou Frou - Breathe In the lilting music and the wry way she uses her voice in this one is captivating.
Frou Frou - It's Good To Be In Love a touch haunting and bittersweet; congratulating an ex on being newly in love rather than crowing about her own. Sort of the talking-to-your-ex perspective of the old 10cc song I'm Not In Love (since covered by Tori Amos and also by Olive, among many many others), if you remember that.
If it tells you anything, those are the first three tracks. LOVE THIS ALBUM.